Total Synthesis of (±)-Maoecrystal V
Gong, Jianxian
Produktnummer:
1869da03758b0c49be9c6f6eaaa16de43e
| Autor: | Gong, Jianxian |
|---|---|
| Themengebiete: | Intramolecular Diels-Alder Reaction Maoecrystal V Natural Product Pinhey Arylation Stereoselective Tetrahydrofuran Oxa-Bridge Skeleton Total Synthesis Wessely Oxidative Dearomatization |
| Veröffentlichungsdatum: | 10.03.2014 |
| EAN: | 9783642543036 |
| Sprache: | Englisch |
| Seitenzahl: | 137 |
| Produktart: | Gebunden |
| Verlag: | Springer Berlin |
Produktinformationen "Total Synthesis of (±)-Maoecrystal V"
In this thesis, the author describes the total synthesis of natural product Maoecrystal V in detail. In the first part of the thesis, the author introduces the research background and reviews the research progress in total synthesis of Maoecrystal V. In the second part, the author develops a novel and concise approach for the stereo selective construction of the tetracyclic model system of Maoecrystal V. The model system is accomplished in 8 steps with 20% yield. In the third part, the author describes the first successful total synthesis of Maoecrystal V and investigates four strategies for constructing the key tetrahydrofuran oxa-bridge skeleton. The total synthesis starts from a known compound and is accomplished in 17 steps with 1.2% yield. The successful total synthesis of Maoecrystal V will contribute to the development of efficient synthetic strategies for natural products and other compounds with complex structures.
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