State-to-State Dynamical Research in the F+H2 Reaction System
Ren, Zefeng
Produktnummer:
18ddf507d7b6744ac089a7ec63e48511de
| Autor: | Ren, Zefeng |
|---|---|
| Themengebiete: | Born-Oppenheimer Approximation Crossed Molecular Beam Scattering Differential Cross Section Feschbach Resonance Hydrogen Atom Rydberg Tagging Time-of-Flight Nonadiabatic Effect Potential Energy Surface Reaction Resonance |
| Veröffentlichungsdatum: | 22.11.2013 |
| EAN: | 9783642397554 |
| Sprache: | Englisch |
| Seitenzahl: | 77 |
| Produktart: | Kartoniert / Broschiert |
| Verlag: | Springer Berlin |
Produktinformationen "State-to-State Dynamical Research in the F+H2 Reaction System"
This thesis addresses two important and also challenging issues in the research of chemical reaction dynamics of F+H2 system. One is to probe the reaction resonance and the other is to determine the extent of the breakdown of the Born-Oppenheimer approximation (BOA) experimentally. The author introduces a state-of-the-art crossed molecular beam-scattering apparatus using a hydrogen atom Rydberg "tagging" time-of-flight method, and presents thorough state-to-state experimental studies to address the above issues. The author also describes the observation of the Feshbach resonance in the F+H2 reaction, a precise measurement of the differential cross section in the F+HD reaction, and validation of a new accurate potential energy surface with spectroscopic accuracy. Moreover, the author determines the reactivity ratio between the ground state F(2P3/2) and the excited state F*(2P1/2) in the F+D2 reaction, and exploits the breakdown of BOA in the low collision energy.
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